Atomic Physics Seminars

Atomic
Monday, November 16, 2020
4:00 PM
Online, Room via Zoom
Note special room.

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"TBA"


Julio Barreiro , UC San Diego
[Host: Peter Schauss]
ABSTRACT:

TBA

Atomic
Monday, March 2, 2020
4:00 PM
Physics Building, Room 204

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"Angular Momentum Coherences in the Ultrafast Dynamics of Isolated Molecules"


Professor Varun Makhija , University of Mary Washington
[Host: Bob Jones]
ABSTRACT:

The development of ultrashort, broadband light pulses in the vacuum ultraviolet enables resonant excitation and probing of the dynamics of isolated molecules. Since the total angular momentum of an isolated system is conserved, broadband excitation necessarily leads to a coherent wavepacket of angular momentum states. Coherences between states of different angular momentum physically manifest as a time varying alignment or orientation of the molecular axis, as well as a much faster variation in the alignment or orientation of the electronic probability distribution, which is synchronized with electronic dynamics occurring in the molecular frame. I will present a direct and selective measurement of this time varying electronic anisotropy, and the potential application of ultrafast scattering probes to this end. I will also briefly discuss the application of purely rotational coherences in the electronic ground state to extract molecular frame information, particularly in the context of photoionization. 

 

 

Special Atomic Seminar


Thursday, January 30, 2020
3:30 PM
Physics Building, Room 204
Note special date.
Note special time.

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ABSTRACT:

The sensitivity of classical Raman spectroscopy methods, such as coherent anti-stokes Raman spectroscopy (CARS) or stimulated Raman spectroscopy (SRS), is ultimately limited by shot-noise from the stimulating fields. I will present a squeezing-enhanced version of Raman spectroscopy that overcomes the shot-noise limit of sensitivity with enhancement of the Raman signal and inherent background suppression, while remaining fully compatible with standard Raman spectroscopy methods. By incorporating the Raman sample between two phase-sensitive parametric amplifiers that squeeze the light along orthogonal quadrature axes, the typical intensity measurement of the Raman response is converted into a quantum-limited, super-sensitive estimation of phase. The resonant Raman response in the sample induces a phase shift to signal-idler frequency-pairs within the fingerprint spectrum of the molecule, resulting in amplification of the resonant Raman signal by the squeezing factor of the parametric amplifiers, whereas the non-resonant background is annihilated by destructive interference. Seeding the interferometer with classical coherent light stimulates the Raman signal further without increasing the background, effectively forming squeezing-enhanced versions of CARS and SRS, where the quantum enhancement is achieved on top of the classical stimulation.

 

References

[1] Yoad Michael, Leon Bello, Michael Rosenbluh and Avi Pe’er, “Squeezing-enhanced Raman Spectroscopy”,  npj  – Quantum Information 5, 81 (2019) .

[2] Y. Shaked, Y. Michael, R. Vered, M. Rosenbluh and A. Pe’er, “Lifting the Bandwidth Limit of Optical Homodyne Measurement,” Nature Communications 9, 609 (2018).

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